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Aerobic and Ligand-Free Manganese-Catalyzed Homocoupling of Arenes or Aryl Halides via in Situ Formation of Aryllithiums

Abstract : Ligand-free manganese-catalyzed homocoupling of arenes or aryl halides can be carried out under aerobic conditions via the in situ formation of the corresponding aryllithiums. A wide range of biaryls and derivatives has been obtained, and a mechanism involving monomeric manganese-oxo complexes has been proposed on the basis of DFT calculations.
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https://hal.archives-ouvertes.fr/hal-02076372
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Submitted on : Thursday, January 7, 2021 - 11:21:20 AM
Last modification on : Tuesday, February 9, 2021 - 11:24:48 AM

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Yujia Liu, Julien Berges, Yassir Zaid, Fouad Ouazzani Chahdi, Arie van der Lee, et al.. Aerobic and Ligand-Free Manganese-Catalyzed Homocoupling of Arenes or Aryl Halides via in Situ Formation of Aryllithiums. Journal of Organic Chemistry, American Chemical Society, 2019, 84 (7), pp.4413-4420. ⟨10.1021/acs.joc.8b02834⟩. ⟨hal-02076372⟩

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